Amide Acetal in Palladium-Catalyzed Allylation with Allylic Alcohols under Neutral Conditions

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초록

A mild and efficient palladium-catalyzed allylation reaction with allylic alcohols is described. The in situ activation of the allylic alcohol is achieved by using N,N-dimethylacetamide dimethyl acetal and a simple palladium catalyst (i.e., Pd(PPh3)(4)). The reaction system does not require acid or base additives or specially designed ligands. In addition to carbon nucleophiles, nitrogen and oxygen nucleophiles can also be used with the allylic alcohol in this transformation.

키워드

alcoholsallylationaminespalladiumsynthetic methodsBAYLIS-HILLMAN ADDUCTSDIRECT AMINATIONSYNTHETIC REACTIONSN-HETEROCYCLESC-OALKYLATIONACIDAMINESSUBSTITUTIONEFFICIENT
제목
Amide Acetal in Palladium-Catalyzed Allylation with Allylic Alcohols under Neutral Conditions
저자
Kwon, YongseokJung, JaehyunKim, Jae HyunKim, Woo-JungKim, Sanghee
DOI
10.1002/ajoc.201600578
발행일
2017-05
유형
Article
저널명
Asian Journal of Organic Chemistry
6
5
페이지
520 ~ 526