Efficient Electrocatalysts for Hydrogen Evolution Reaction Using Heteroatom-Doped MXene Nanosheet
  • Tekalgne, Mahider Asmare
  • Do, Ha Huu
  • Nguyen, Tuan Van
  • Le, Quyet Van
  • An, Jusung
  • ... Ahn, Sang Hyun
  • 외 4명
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초록

It is crucial to develop a low-cost hybrid electrocatalysts for hydrogen production. Due to their layered structure and strong electrical conductivity, MXene-based materials have been lately used more and more in energy storage devices. Herein, heteroatom- (boron and sulfur-) doped MXene (B, S-Ti3C2Tx) nanosheets are developed as efficient electrocatalysts for the hydrogen evolution reaction (HER). The synthesized B, S-Ti3C2Tx has a large surface area and exhibits excellent electrocatalytic activity in acidic media. The prepared B, S-2-Ti3C2Tx catalyst exhibits a low overpotential of -110 mV vs. reversible hydrogen electrode for the HER and a low Tafel slope of similar to 54 mV dec(-1). Furthermore, B, S-2-Ti3C2Tx shows a double-layer capacitance of 1.05 mF/cm(2) and maintains a steady catalytic activity for the HER for over 1000 cycles.

키워드

RAY PHOTOELECTRON-SPECTROSCOPYBORONINTERCALATIONCATALYSTSPHOSPHIDEHYBRIDSITESMOS2TI2C
제목
Efficient Electrocatalysts for Hydrogen Evolution Reaction Using Heteroatom-Doped MXene Nanosheet
저자
Tekalgne, Mahider AsmareDo, Ha HuuNguyen, Tuan VanLe, Quyet VanAn, JusungHong, Sung HyunAhn, Sang HyunKang, HeeminKim, Jong SeungKim, Soo Young
DOI
10.1155/2023/8980888
발행일
2023-05
유형
Article
저널명
International Journal of Energy Research
2023

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