SYNTHESIS OF DILITHIUM ALPHA,OMEGA-DISULFONATED POLYSTYRENE BY ANIONIC-POLYMERIZATION

  • KIM, Jungahn
  • LEE, MiKyung
  • RYU, Chang-Yeol
  • LEE, Jonghwi
  • HWANG, Seung Sang
  • 외 7명
Citations

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초록

The chain-end sulfonation of alpha,omega-dilithiopolystyrene prepared by lithium naphthalenide as a difunctional initiator using 1,3-propanesultone was studied by the characterization methodologies such as acid/base titration, colorimetric method using methylene blue, two-phase titration with Hyamine 1622, size exclusion chromatographic analysis infrared, and H-1 NMR spectroscopic analysis. The reactivity modification of alpha,omega-dilithiopolystyrene through the end-capping with 1,1-diphenylethylene prior to the sulfoalkylation in benzene-tetrahydrofuran (THF) (10:1, v/v) at 25-degrees-C with excess 1,3-propanesultone is suggested as a useful method for the preparation of the corresponding dilithium alpha,omega-disulfonated polystyrene in relatively high yield based on the results from the acid/base titration (>85%).

키워드

ALPHA,OMEGA-DILITHIOPOLYSTYRENEDIFUNCTIONAL INITIATORALPHA,OMEGA-BIS(1-LITHIO-1,1-DIPHENYLETHYL)POLYSTYRENESULFOALKYLATION1,3-PROPANESULTONEDILITHIUMALPHA,OMEGA-DISULFONATED POLYSTYRENESIZE EXCLUSION CHROMATOGRAPHYHALATO-TELECHELIC POLYMERSIONOMERSLITHIUM
제목
SYNTHESIS OF DILITHIUM ALPHA,OMEGA-DISULFONATED POLYSTYRENE BY ANIONIC-POLYMERIZATION
저자
KIM, JungahnLEE, MiKyungRYU, Chang-YeolLEE, JonghwiHWANG, Seung SangPARK, Tae SukKIM, Kwang UngYOON, Hye SungAHN, Byeong InCHAR, KookheonRYU, Joo HanQUIRK, Roderic P.
DOI
10.1295/polymj.26.1111
발행일
1994-01
유형
Article
저널명
Polymer Journal
26
10
페이지
1111 ~ 1117